Ni/Hierarchical Zeolites Derived from Zeolites@Layered Double Hydroxides (LDHs) Composites for Furfural Hydrogenation
Narasiri Maineawklang
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Conceptualization (lead), Formal analysis (lead), Investigation (lead), Writing - original draft (lead)
Search for more papers by this authorDr. Ploychanok Iadrat
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting), Writing - original draft (supporting)
Search for more papers by this authorDr. Peerapol Pornsetmetakul
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting)
Search for more papers by this authorAnittha Prasertsab
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting)
Search for more papers by this authorPeeranat Chaipornchalerm
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Saros Salakhum
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Supakorn Tantisriyanurak
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Chadatip Rodaum
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorCorresponding Author
Assoc. Prof. Dr. Chularat Wattanakit
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Conceptualization (lead), Resources (lead), Supervision (lead), Writing - review & editing (lead)
Search for more papers by this authorNarasiri Maineawklang
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Conceptualization (lead), Formal analysis (lead), Investigation (lead), Writing - original draft (lead)
Search for more papers by this authorDr. Ploychanok Iadrat
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting), Writing - original draft (supporting)
Search for more papers by this authorDr. Peerapol Pornsetmetakul
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting)
Search for more papers by this authorAnittha Prasertsab
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting), Methodology (supporting)
Search for more papers by this authorPeeranat Chaipornchalerm
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Saros Salakhum
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Supakorn Tantisriyanurak
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorDr. Chadatip Rodaum
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Investigation (supporting)
Search for more papers by this authorCorresponding Author
Assoc. Prof. Dr. Chularat Wattanakit
Department of Chemical and Biomolecular Engineering, School of Energy Science and Engineering, Vidyasirimedhi Institute of Science and Technology, Rayong, 21210 Thailand
Contribution: Conceptualization (lead), Resources (lead), Supervision (lead), Writing - review & editing (lead)
Search for more papers by this authorAbstract
Furfural hydrogenation is one of the most important reactions for the transformation of biomass-derived resources into high value-added chemicals. To achieve a highly efficient catalytic activity of the reaction, catalysts with a high dispersion of metal nanoparticles (NPs) on solid supports are required. However, the development of highly efficient and stable catalysts is still challenging. Herein, the highly dispersed nickel nanoparticles (Ni NPs) supported on the hierarchical ZSM-5 nanosheets (Z5-NS) derived from the hierarchical ZSM-5 nanosheets@NiAl-layered double hydroxides (LDHs) composites were successfully fabricated. Remarkably, the fabricated Z5-NS/Ni catalyst exhibited a high furfural conversion of 85 % with a yield of furfuryl alcohol of 60 %. This work illustrates the fabrication of highly metal dispersed on solid supports with high metal loading, which can enhance the catalytic performances in the hydrogenation of biomass-derived compounds.
Conflict of interests
The authors declare no conflict of interest.
Open Research
Data Availability Statement
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Supporting Information
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